PERMEATION SETUP

Single gas (mono-component) permeation experiments are performed at 25 ºC (inside a thermostatic chamber) in a home-made permeation set-up, as shown in Figure 1.

Figure 1 - Single gas permeation setup
Figure 1. Single gas (mono-component) permeation setup.

Mixed gas (multi-component) permeation experiments are performed at 25 ºC (inside a thermostatic chamber) in a home-made permeation set-up, as shown in Figure 2.

Figure 2 - Mixed gas permeation setup
Figure 2. Mixed gas (multi-component) permeation setup.

Before the permeation experiments, membranes are glued to a steel O-ring support with an epoxy glue (Araldite® Standard) – Figure 3.

Figure 3 - Membrane glued to steel O-ring
Figure 3. Membranes glued to a steel O-ring support with epoxy glue.

After, the epoxy glue cured for approximately 6 hours and then membranes are placed inside the membrane cell – Figure 4. The entire system is then evacuated until a pressure of ca. 0.01 bar. After that, a feed pressure of 1 bar is fed to the cell.

Figure 4 - Membrane placed inside the membrane cell
Figure 4. Membrane placed inside the membrane cell.

The permeability of the membranes is computed from the time derivative of the permeating pressure. The permeability of a membrane, \( P_i \), is calculated from the equation:

Equation

where \( \delta \) is the membrane thickness (determined with a high accuracy digital micrometer, Mitutoyo MDH-25M), \( V_p \) is the volume of the permeate tank, \( \nu_M \) is the molar volume of the gas at normal conditions, \( R \) is the universal gas constant, \( T \) is the absolute temperature, \( p_f \) and \( p_p \) are the feed and the permeate pressure, respectively, and \( t \) is the time.